Experiments are reported on helical plasma equilibrium and stability in the Scyllac toroidal θ-pinch sectors (120°) which have major radii of 2.375 and 4.0 m with coil arc lengths of 5.0 and 8.4 m, respectively. In these experiments the outward toroidal drift force was compensated by a combination of ℓ = 1 helical and ℓ = 0 bumpy fields which are generated by shaping the inner surface of the compression coil or by driven ℓ = 1 windings. Time-resolved measurements were made of the gross plasma-column motion, the plasma radius, the magnetic flux excluded by the plasma, the external magnetic field, the plasma density, the electron and ion temperatures, and the plasma β at axial locations of minimum and maximum plasma radius. These data are used to study the approach to the theoretically predicted toroidal equilibrium (including axial pressure equilibrium). The plasma column remained in stable equilibrium for 7 – 10 μs in the 8-m sector compared with 4 – 7 μs in the 5-m experiment, at which times the onset of a terminating m = 1, k ≈ 0 sideways motion occurred. The results show that the plasma achieved axial pressure equilibrium (nkT = const) in 4 – 6 μs, while maintaining equilibrium in the toroidal plane for 10 μs or longer. The measurements of the plasma radius, β and magnetic field in the various experiments have confirmed in detail the stable toroidal equilibrium observed in the streak photographs during the first 4-10 μs of the discharge. The observed toroidal equilibria of the high-β, θ-pinch plasma are in quantitative agreement with MHD sharp-boundary theory and confirm the theoretical scaling of the equilibrium field between the 5-m and the 8-m sector experiments.