The Chern-Simons functionals built from various connections determined by the initial data hµ
,
µ
on a 3-manifold
are investigated. First it is shown that for asymptotically flat data sets the logarithmic fall off for hµ
and r
µ
is the necessary and sufficient condition for the existence of these functionals. The functional Y(k
,l
)
, built in the vector bundle corresponding to the irreducible representation of SL
(2,
) labelled by (k
,l
), is shown to be determined by the Ashtekar-Chern-Simons functional and its complex conjugate. Y(k
,l
)is conformally invariant precisely in the l= k(i.e. tensor) representations. An unexpected connection with twistor theory is found: Y(k
,k
)can be written as the Chern-Simons functional built from the 3-surface twistor connection, and the not identically vanishing spinor parts of the 3-surface twistor curvature are given by the variational derivatives of Y(k
,k
)with respect to hµ
and
µ
. The time derivative
(k
,k
)of Y(k
,k
)is another global conformal invariant of the initial data set, and for vanishing
(k
,k
)
, in particular for all Petrov III and N spacetimes, the Chern-Simons functional is a conformal invariant of the whole spacetime.