Abstract
We identify ambiguities in the available frameworks for defining quantum, classical, and total correlations as measured by discord-like quantifiers. More specifically, we determine situations for which either classical or quantum correlations are not uniquely defined due to degeneracies arising from the optimization procedure over the state space. In order to remove such degeneracies, we introduce a general approach where correlations are independently defined, escaping therefore from a degenerate subspace. As an illustration, we analyze the trace-norm geometric quantum discord for two-qubit Bell-diagonal states.
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Introduction
Quantum correlations are widely recognized as a resource for quantum information tasks [1]. In this scenario, entanglement plays a special role for applications in quantum computation and quantum communication [2]. On the other hand, it is now known that, even in the absence of entanglement, it is possible to achieve some quantum advantage, such as in protocols for work extraction via Maxwell's demons [3], metrology [4,5], entanglement distribution [6–10], quantum state merging [11], among others. The source for the quantum power of such tasks can be attributed to more general quantum correlations, as measured by quantum discord [12]. Such correlations can be suitably applied to make quantum systems supersede their classical counterparts.
Quantum information science has then motivated the development of a general theory of quantum, classical, and total correlations in physical systems. In this context, quantum discord has been originally introduced by Ollivier and Zurek [12] as an entropic measure of quantum correlation in a bipartite system, which arises as a difference between the total correlation (as measured by the mutual information) before and after a local measurement is performed over one of the subsystems. In addition, a number of discord-like measures have also appeared through a geometric formulation, which are based, e.g., on the relative entropy [13,14], Hilbert-Schmidt norm [15,16], trace norm [17,18], and Bures norm [19,20]. All of these distinct versions can be generally described by a unified framework in terms of a distance function. Here, the term distance will be generically used as a measure of distinguishability between two density operators (not necessarily a proper distance). Then, a correlation measure (either classical, quantum, or total) can be obtained by computing the distance function associated with a state ρ and a related classical or product state.
By focusing on the quantumness of ρ, we typically optimize the distance function via a pre-selected strategy over classical states, which leads to a unique value for the quantum correlation. We then compute the distance function between the optimal classical state and a product state (or a measured product state) to obtain the classical correlation. However, as we will explicitly show in this work, there may be more than a single optimal classical state. This set of optimal classical states, which are degenerate in the sense that they provide the same value for the quantum correlation, can lead to a nonunique (multivalued) classical correlation. Therefore, there is an ambiguity in the definition of the classical correlation. This result is independent of the distance function adopted, affecting all the discord-like measures (see, e.g., a brief discussion for the specific cases of the Bures distance [20] and the measurement-induced disturbance [21]). Moreover, by choosing first to optimize the distance function for the classical correlation, the nonuniqueness will be moved to the subsequent optimization of the quantum correlation. In order to remove those degeneracies for both classical and quantum correlations, we propose a general strategy based on an independent optimization procedure. As will be shown, this will lead to the uniqueness of the distance functions, providing a consistent theory of correlations.
Distance functions
Discord-like measures of quantum correlation are typically devised to quantify the disturbance of quantum states under local measurements. In this sense, even separable states may exhibit quantumness. Quantum correlation is part of the total correlation exhibited by a quantum state, which is also composed by the classical correlation. Proposals of bona fide measures for quantum, classical, and total correlations are expected to obey a set of fundamental criteria [1,22]: i) product states have no correlations, ii) all correlations are invariant under local unitary operations, iii) all correlations are non-negative, iv) total correlations are nonincreasing under local operations, and v) classical states have no quantum correlations. Moreover, an extra assumption has been recently taken as necessary [17,23–25]: vi) quantum correlations are nonincreasing under local operations over unmeasured subsystems. This set of fundamental criteria has been used as a guide to validate correlation measures. In the following subsections, we will describe possible frameworks to unify correlation definitions, which can be established by either measurement-based or measurement-independent approaches.
Measurement-based approach
In the general method presented by Brodutch and Modi [1,22] discord-like measures of quantum, classical, and total correlations of an n-partite system in a state ρ are respectively defined by
where represents the product of the local marginals of ρ: the state you would have if all the correlations between the n parts were erased. denotes a real-valued function that vanishes for , and is a classical state emerging from a measurement on ρ chosen according to a pre-selected strategy. In eq. (2), is defined as a measurement over the product of the marginals of ρ [1]. Instead, an alternative definition would be to first measure ρ and then take the product of the marginals of , as adopted in ref. [22]. For an n-partite system , the classical states assume the form , where pi is a joint probability distribution and is a set of orthogonal projectors for subsystem Aj.
It can be shown that a number of correlation quantifiers are compatible with the fundamental criteria of correlations listed above. Explicit examples in the class of entropic measures include the mutual information , the conditional entropy , and the von Neumann entropy . In the class of geometric measures, one has the Schatten 1-norm (trace norm) , with , among others. Concerning , it is usually defined as a positive operator-valued measure (POVM) over one or more of the subsystems such that: a) it minimizes the quantum correlation or b) it maximizes the classical correlation.
Measurement-independent approach
A measurement-independent approach has also been introduced for different discord-like measures [13,16,20,26]. In terms of the generalized function K, we can express the quantum, classical, and total correlations in this approach respectively by
For the evaluation of the function K, denotes the classical state closest to ρ among a pre-selected set of classical states , whereas and represent the product states closest to and ρ, respectively. In comparison with the measurement-based formalism, the optimization of eqs. (4)–(6) may lead to and even in the case (which occurs for [26,27]). On the other hand, both approaches are equivalent in terms of obeying the fundamental criteria.
Ambiguities
Both the measurement-based and the measurement-independent approaches yield well-defined frameworks as long as the optimized classical state involved (either or ) is unique for any given ρ. However, this assumption is not true in general. Degenerate classical states, which lead to a single value of quantum correlation but nonunique values for the classical correlation (and vice versa in the case of the measurement-based framework), are often present in the optimization performed over state space. As an example, fig. 1 provides a sketch of such degeneracies in the measurement-independent formalism.
As an explicit illustration of these ambiguities, let us consider a function K based on the Schatten 1-norm and a classical state emerging from a projective measurement over one qubit of a two-qubit system so that minimizes the quantum correlation Q. Then, we have
where represent the eigenvalues of the Hermitian operator and are projection operators, being the identity matrix, a vector formed by Pauli matrices, and a unitary vector that minimizes eq. (7). In this scenario, Q is equivalent to the 1-norm geometric quantum discord, which is defined by with denoting the classical-quantum state closest to ρ [17,18]. In particular, by taking the two-qubit system as described by a Bell-diagonal state, its density operator reads
where is a three-dimensional vector composed by the correlation functions ( and z). In this case, the optimized classical state, the product of the local marginals of , and the product state closest to the optimized classical state have been computed in refs. [26,27], yielding
In eqs. (10)–(12), is such that (maximum element of the set ), whereas and . Defining and (intermediate element of the set ), eqs. (10)–(12) lead to the following expressions for the quantum and classical correlations [26,27]:
where Q, C, , and are obtained from eqs. (1), (2), (4), and (5), respectively, with the distance function K given in terms of the Schatten 1-norm. Now, let us prove that the optimized classical state in eq. (10) is nonunique, implying there are multiple values for the classical correlations. In order to provide a concrete example of ambiguity, let us consider a restricted class of Bell-diagonal states , which is given by
where the correlation vector is , with c > 0. In this case, the possible four eigenvalues of the operator are given by , where . So, taking into account these eigenvalues in eq. (7), we obtain that the quantum correlation reads
with an arbitrary unitary vector. This result is in agreement with eq. (13) applied to the state described in eq. (16). However, its independence of reveals the existence of an infinity number of optimized classical states associated with a unique value of . Such degeneracy implies into a continuum of inequivalent values for the classical correlation. Indeed, the eigenvalues of are given by , where . This leads to
with . Note that eq. (18) agrees with eq. (14) applied to the state only in the case , i.e., when lies on the xy-plane. This includes the particular solutions or associated with the classical state in eq. (10). The maximal discrepancy occurs for , where the classical correlation in eq. (18) goes to zero. A schematic picture of this situation is shown in fig. 2. Concerning the measurement-independent framework, we find
where we have used the relations , , and into the definitions of quantum and classical correlations. From eqs. (10) and (15), we can derive that
whereas from eqs. (20) and (18) we obtain
This variation of for distinct choices of is sufficient to show that the nonuniqueness also affects the measurement-independent approach.
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Standard imageNew framework
As long as the fundamental criteria of reasonable correlation measures are satisfied, it is plausible to add auxiliary strategies to the previous frameworks in order to overcome ambiguities originated from the degeneracies. As an example, we could adopt the following modified strategy (see subsect. "Measurement-based approach" for the original strategy): ) maximize the classical correlation or ) minimize the quantum correlation over the degenerate subspace. However, depending on the distance function K and for general quantum states, it may not be a trivial task to find out the degenerate subspace as well as to optimize over the degenerate classical states. Here, we propose a new framework based on the measurement-based approach, which has the advantage of avoiding extra optimization over the degenerate subspace. In this new framework, the quantum, classical, and total correlations are independently obtained from
where and are classical states that minimizes and maximizes within a pre-established set of measurements (e.g., orthogonal projective measurements), respectively. In this approach, degeneracies in or are irrelevant, being it sufficient to find out a unique solution for each optimal measurement. More specifically, and are independently optimized, with no direct connection between them. As an application, let us assume , , and , i.e., orthogonal projective measurements, where and denote the unitary vectors that minimize and maximize , respectively. From previous analysis, it follows that or , with , such that
Concerning the evaluation of the classical correlation, we find , where we have defined with and . These eigenvalues lead to
where maximizes eq. (27) under the conditions and . By defining , , , , , and , where max, int, and min, denote maximum, intermediate, and minimum, respectively, we can write
with
Then, isolating in terms of u0 and in eq. (29) and inserting the resulting expression in eq. (28), we obtain
where we have used the relations , , , and . Evidently, the maximum value of the function can be achieved for , , and , i.e., for . Consequently, . Thus, it follows that
Remarkably, the framework introduced here and the measurement-based approach with given by eq. (10) (see ref. [27]) lead to the same expressions for the correlations in the particular case of the Bell-diagonal states, even though inequivalent results may appear for more general states. Furthermore, it is also important to emphasize that the alternative strategy of further optimization over the degenerate subspace (instead of independent optimization of Q and C) also provides the same results. Indeed, since we have shown that there is at least one optimized classical state in common for and , given by eq. (10), then eqs. (26) and (31) can also be obtained from the measurement-based formalism by assuming strategy a) in combination with ) or b) followed by .
Conclusions
In summary, we have identified ambiguities in the definition of either classical or quantum correlations, which potentially affect all the approaches used to define discord-like measures. Moreover, we have proposed a new framework to avoid such ambiguities by independent optimization of the correlation functions. These results are relevant for a consistent correlation theory and for practical applications of correlation measures, such as in quantum many-body systems [28,29], in the emergence of the pointer basis in open quantum systems [30,31], etc. As future challenges, it remains the application of the proposed framework for states more general than the Bell-diagonal qubit-qubit states, the investigation of its robustness against decoherence, and possible relevance in quantum information tasks.
Acknowledgments
We thank Gerardo Adesso for useful discussions. This work is supported by the Brazilian agencies CNPq, CAPES, FAPERJ, and the Brazilian National Institute for Science and Technology of Quantum Information (INCT-IQ).