Relaxational dynamics of polar nanodomains in Sr1 − xCaxTiO3 x = 0.002

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1997 EDP Sciences
, , Citation W. Kleemann et al 1997 EPL 37 145 DOI 10.1209/epl/i1997-00124-7

0295-5075/37/2/145

Abstract

The dielectric permittivity of Sr1 − xCaxTiO3, x = 0.002, measured at frequencies 10−3f ⩽ 107 Hz and temperatures 1.5 ⩽ T ⩽ 15 K, exhibits enhanced loss, ε''(f), on its low-f slope. This contrasts with conventional glassy dynamics and is attributed to dynamic heterogeneity involving thermally activated relaxation of dynamically coupled mesoscopic domains. Crossover into non-activated dynamics occurs at very low f as corroborated by temporal relaxation studies of the field-induced polarization P. Below T ≈ 3 K athermal quantum tunneling starts to dominate both ε''(f) and P(t).

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10.1209/epl/i1997-00124-7