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Delocalization of Wannier-Stark ladders by phonons: Tunneling and stretched polarons

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2002 EDP Sciences
, , Citation W. Zhang et al 2002 EPL 58 857 DOI 10.1209/epl/i2002-00453-y

0295-5075/58/6/857

Abstract

We study the coherent dynamics of a Holstein polaron in strong electric fields. A detailed analytical and numerical analysis shows that even for small hopping constant and weak electron-phonon interaction, polaron states can become delocalized if a resonance condition develops between the original Wannier-Stark states and the phonon modes, yielding both tunneling and "stretched" polarons. The unusual stretched polarons are characterized by a phonon cloud that trails the electron, instead of accompanying it. In general, our novel approach allows us to show that the polaron spectrum has a complex nearly fractal structure, due to the coherent coupling between states in the Cayley tree which describes the relevant Hilbert space. The eigenstates of a finite ladder are analyzed in terms of the observable tunneling and optical properties of the system.

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10.1209/epl/i2002-00453-y