Mass-dependent isotopic fractionation of a solid tin under a strong gravitational field

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Published 2 April 2009 Europhysics Letters Association
, , Citation Takahito Osawa et al 2009 EPL 85 64001 DOI 10.1209/0295-5075/85/64001

0295-5075/85/6/64001

Abstract

Pure tin metals were centrifuged at 1 × 106g and at 220°C for 100 hours, at 0.40 × 106g at 220–230°C for 24 hours, and at 0.25 × 106g at 220°C for 24 hours. Their isotopic compositions were measured by a secondary ion mass spectrometer (SIMS). 116Sn/120Sn and 124Sn/120Sn ratios of the 1.02 × 106g sample were considerably different than the initial compositions, and the magnitude of isotopic fractionation reached 2.6 ± 0.1%. A three-isotope diagram of 116Sn/120Sn vs.124Sn/120Sn shows conclusively that isotopic fractionation caused by a gravitational field depended only on the isotopic mass.

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10.1209/0295-5075/85/64001