Multiphoton dynamics and resonance lineshapes in three-level systems: many-mode Floquet treatment

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, , Citation Kwanghsi Wang et al 1985 J. Phys. B: Atom. Mol. Phys. 18 4539 DOI 10.1088/0022-3700/18/23/008

0022-3700/18/23/4539

Abstract

The authors present an exact treatment of two- and multiquantum transitions in three-level systems driven by two intense linearly polarised monochromatic fields based on the semiclassical many-mode Floquet theory developed recently. Further they extend the almost degenerate perturbation theory of Salwen (1955-6) to the two-mode Floquet Hamiltonian and obtain approximate analytical formulae for multiphoton transition probabilities, resonance bichromatic shifts and widths, and absorption lineshapes beyond the conventional rotating-wave approximation (RWA). Detailed comparison of the analytical, the RWA, and the exact results is given. Several novel features of multiphoton lineshape characteristics are pointed out.

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10.1088/0022-3700/18/23/008